The best replacement for merino is cashmere.

The best alternatives to merino are rated as following:
★★★★★  cashmere
★★★  lambswool
★★★  alpaca
★  capilene
★  alpaca wool
★  cotton cashmere
★  worsted wool
★  smartwool
  polyprop
  lambs wool
  merino
  mohair
  coolmax
  polypro
  angora

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Google Trends

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merino
cashmere
lambswool