The best replacement for jigglypuff is clefairy.

The best alternatives to jigglypuff are rated as following:
★★★★★  clefairy
★★★★  kirby
★★★  marth
★★  wigglytuff
★★  gengar
★  meloetta
★  meta knight
★  clefairy fire red
  rattata
  young link
  meowth

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No companions for jigglypuff have been suggested so far.
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Google Trends

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jigglypuff
clefairy
kirby