The best replacement for cointreau is triple sec.

The best alternatives to cointreau are rated as following:
★★★★★  triple sec
★★★★  grand marnier
★★  curacao
★★  grand marnier margarita
★  patron citronge
★  combier
★  triple sec margarita
★  citronge
★  triple sec cosmopolitan
  gran gala
  drambuie
  grand mariner
  orange curacao
  grand gala
  gran marnier
  campari
  grand marnier liquor
  dekuyper
  triple sec cocktail
  o3
  hiram walker
  aperol

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Google Trends

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cointreau
triple sec
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