The best replacement for barbiturates is benzodiazepines.

The best alternatives to barbiturates are rated as following:
★★★★★  benzodiazepines
★★  opiates
★★  narcotics
★  non barbiturates
★  benzodiazepine
★  benzos
  opioids
  barbiturates

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Google Trends

Scale is based on the average worldwide traffic of barbiturates in all years. Click on graph for more.
barbiturates
benzodiazepines
opiates