The best replacement for megabus is greyhound.

The best alternatives to megabus are rated as following:
★★★★★  greyhound
★★★  boltbus
★★★  amtrak
★★  bolt
★★  national express
★  greyhound express
★  peter pan
★  gotobus
★  bolt bus
★  idbus
★  go bus
★  greyhound better
★  eurolines
  fung wah
  greyhound bus
  bolt better
  national express better

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Google Trends

Scale is based on the average worldwide traffic of megabus in all years. Click on graph for more.
megabus
greyhound
boltbus